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\u003Cdiv class=\u0022pane-content\u0022\u003E\n \u003Cdiv class=\u0022elements-frag-data highwire-markup\u0022 id=\u0022fig-data\u0022\u003E\u003Cdiv id=\u0022fig-data-figures\u0022 class=\u0022group frag-figure\u0022\u003E\u003Cdiv class=\u0022fig-data-title-jump clearfix\u0022\u003E\u003Ch3 class=\u0022fig-data-group-title\u0022\u003EFigures\u003C\/h3\u003E\u003Cdiv class=\u0022fig-data-jump-links\u0022\u003E\u003C\/div\u003E\u003C\/div\u003E\u003Cdiv class=\u0022item-list\u0022\u003E\u003Cul class=\u0022fig-data-list clearfix\u0022 id=\u0022fragments-fig\u0022\u003E\u003Cli class=\u0022first\u0022\u003E\u003Cdiv class=\u0022element-fig-data clearfix figure-caption\u0022\u003E\u003Cdiv class=\u0022highwire-markup\u0022\u003E\u003Cdiv xmlns=\u0022http:\/\/www.w3.org\/1999\/xhtml\u0022 id=\u0022content-block-markup\u0022 xmlns:xhtml=\u0022http:\/\/www.w3.org\/1999\/xhtml\u0022\u003E\u003Cdiv class=\u0022fig-expansion type-featured \u0022 id=\u0022F1\u0022\u003E\u003Cspan class=\u0022highwire-journal-article-marker-start\u0022\u003E\u003C\/span\u003E\u003Cdiv class=\u0022highwire-figure\u0022\u003E\u003Cdiv class=\u0022fig-inline-img-wrapper\u0022\u003E\u003Cdiv class=\u0022fig-inline-img\u0022\u003E\u003Ca href=\u0022https:\/\/广东快乐十分投注下载 www.hmclip.net\/content\/pnas\/116\/12\/5383\/F1.large.jpg?width=800\u0026amp;height=600\u0026amp;carousel=1\u0022 title=\u0022(A) Simplified diagram of the SRS process, which induces correlations of spectral components at frequencies \u0026#x3C9; and \u0026#x3C9; \u0026#xB1; \u0026#x3A9;. The shaped pulses can be divided into a coherent component (blue) and a noisy tail (green). (B) The experimental apparatus. (C and D) Pearson correlation plots for all pairs of frequencies within the excitation spectrum (C) after the pulse shaper, and (D) after the quartz sample. (E) Spontaneous Raman spectrum of quartz (14), matching the positions of the features in the covariance map in D.\u0022 class=\u0022highwire-fragment fragment-images colorbox-load\u0022 rel=\u0022gallery-fragment-images-1831827155\u0022 data-figure-caption=\u0022\u0026lt;div class=\u0026quot;highwire-markup\u0026quot;\u0026gt;\u0026lt;div xmlns=\u0026quot;http:\/\/www.w3.org\/1999\/xhtml\u0026quot;\u0026gt;(\u0026lt;em\u0026gt;A\u0026lt;\/em\u0026gt;) Simplified diagram of the SRS process, which induces correlations of spectral components at frequencies \u0026#x3C9; and \u0026#x3C9; \u0026#xB1; \u0026#x3A9;. The shaped pulses can be divided into a coherent component (blue) and a noisy tail (green). (\u0026lt;em\u0026gt;B\u0026lt;\/em\u0026gt;) The experimental apparatus. (\u0026lt;em\u0026gt;C\u0026lt;\/em\u0026gt; and \u0026lt;em\u0026gt;D\u0026lt;\/em\u0026gt;) Pearson correlation plots for all pairs of frequencies within the excitation spectrum (\u0026lt;em\u0026gt;C\u0026lt;\/em\u0026gt;) after the pulse shaper, and (\u0026lt;em\u0026gt;D\u0026lt;\/em\u0026gt;) after the quartz sample. (\u0026lt;em\u0026gt;E\u0026lt;\/em\u0026gt;) Spontaneous Raman spectrum of quartz (14), matching the positions of the features in the covariance map in \u0026lt;em\u0026gt;D\u0026lt;\/em\u0026gt;.\u0026lt;\/div\u0026gt;\u0026lt;\/div\u0026gt;\u0022 data-icon-position=\u0022\u0022 data-hide-link-title=\u00220\u0022\u003E\u003Cspan class=\u0022hw-responsive-img\u0022\u003E\u003Cimg class=\u0022highwire-fragment fragment-image lazyload\u0022 alt=\u0022Fig. 1.\u0022 src=\u0022data:image\/gif;base64,R0lGODlhAQABAIAAAAAAAP\/\/\/yH5BAEAAAAALAAAAAABAAEAAAIBRAA7\u0022 data-src=\u0022https:\/\/广东快乐十分投注下载 www.hmclip.net\/content\/pnas\/116\/12\/5383\/F1.medium.gif\u0022 width=\u0022440\u0022 height=\u0022159\u0022\/\u003E\u003Cnoscript\u003E\u003Cimg class=\u0022highwire-fragment fragment-image\u0022 alt=\u0022Fig. 1.\u0022 src=\u0022https:\/\/广东快乐十分投注下载 www.hmclip.net\/content\/pnas\/116\/12\/5383\/F1.medium.gif\u0022 width=\u0022440\u0022 height=\u0022159\u0022\/\u003E\u003C\/noscript\u003E\u003C\/span\u003E\u003C\/a\u003E\u003C\/div\u003E\u003C\/div\u003E\u003Cul class=\u0022highwire-figure-links inline\u0022\u003E\u003Cli class=\u0022download-fig first\u0022\u003E\u003Ca href=\u0022https:\/\/广东快乐十分投注下载 www.hmclip.net\/content\/pnas\/116\/12\/5383\/F1.large.jpg?download=true\u0022 class=\u0022highwire-figure-link highwire-figure-link-download\u0022 title=\u0022Download Fig. 1.\u0022 data-icon-position=\u0022\u0022 data-hide-link-title=\u00220\u0022\u003EDownload figure\u003C\/a\u003E\u003C\/li\u003E\n\u003Cli class=\u0022new-tab\u0022\u003E\u003Ca href=\u0022https:\/\/广东快乐十分投注下载 www.hmclip.net\/content\/pnas\/116\/12\/5383\/F1.large.jpg\u0022 class=\u0022highwire-figure-link highwire-figure-link-newtab\u0022 target=\u0022_blank\u0022 data-icon-position=\u0022\u0022 data-hide-link-title=\u00220\u0022\u003EOpen in new tab\u003C\/a\u003E\u003C\/li\u003E\n\u003Cli class=\u0022download-ppt last\u0022\u003E\u003Ca href=\u0022\/highwire\/powerpoint\/855270\u0022 class=\u0022highwire-figure-link highwire-figure-link-ppt\u0022 data-icon-position=\u0022\u0022 data-hide-link-title=\u00220\u0022\u003EDownload powerpoint\u003C\/a\u003E\u003C\/li\u003E\n\u003C\/ul\u003E\u003C\/div\u003E\u003Cdiv class=\u0022fig-caption\u0022 xmlns:xhtml=\u0022http:\/\/www.w3.org\/1999\/xhtml\u0022\u003E\u003Cspan class=\u0022fig-label\u0022\u003EFig. 1.\u003C\/span\u003E \u003Cp id=\u0022p-15\u0022\u003E(\u003Cem\u003EA\u003C\/em\u003E) Simplified diagram of the SRS process, which induces correlations of spectral components at frequencies \u03c9 and \u03c9 \u00b1 \u03a9. The shaped pulses can be divided into a coherent component (blue) and a noisy tail (green). (\u003Cem\u003EB\u003C\/em\u003E) The experimental apparatus. (\u003Cem\u003EC\u003C\/em\u003E and \u003Cem\u003ED\u003C\/em\u003E) Pearson correlation plots for all pairs of frequencies within the excitation spectrum (\u003Cem\u003EC\u003C\/em\u003E) after the pulse shaper, and (\u003Cem\u003ED\u003C\/em\u003E) after the quartz sample. (\u003Cem\u003EE\u003C\/em\u003E) Spontaneous Raman spectrum of quartz (\u003Cspan id=\u0022xref-ref-14-2\u0022 class=\u0022xref-bibr\u0022\u003E14\u003C\/span\u003E), matching the positions of the features in the covariance map in \u003Cem\u003ED\u003C\/em\u003E.\u003C\/p\u003E\u003Cdiv class=\u0022sb-div caption-clear\u0022\u003E\u003C\/div\u003E\u003C\/div\u003E\u003Cspan class=\u0022highwire-journal-article-marker-end\u0022\u003E\u003C\/span\u003E\u003C\/div\u003E\u003Cspan id=\u0022related-urls\u0022\u003E\u003C\/span\u003E\u003C\/div\u003E\u003C\/div\u003E\u003C\/div\u003E\u003C\/li\u003E\n\u003Cli class=\u0022last\u0022\u003E\u003Cdiv class=\u0022element-fig-data clearfix figure-caption\u0022\u003E\u003Cdiv class=\u0022highwire-markup\u0022\u003E\u003Cdiv xmlns=\u0022http:\/\/www.w3.org\/1999\/xhtml\u0022 id=\u0022content-block-markup\u0022 xmlns:xhtml=\u0022http:\/\/www.w3.org\/1999\/xhtml\u0022\u003E\u003Cdiv class=\u0022fig-expansion type-figure \u0022 id=\u0022F2\u0022\u003E\u003Cspan class=\u0022highwire-journal-article-marker-start\u0022\u003E\u003C\/span\u003E\u003Cdiv class=\u0022highwire-figure\u0022\u003E\u003Cdiv class=\u0022fig-inline-img-wrapper\u0022\u003E\u003Cdiv class=\u0022fig-inline-img\u0022\u003E\u003Ca href=\u0022https:\/\/广东快乐十分投注下载 www.hmclip.net\/content\/pnas\/116\/12\/5383\/F2.large.jpg?width=800\u0026amp;height=600\u0026amp;carousel=1\u0022 title=\u0022Covariance maps recorded in \u0026#x3B1;-quartz by applying uniform phase noise to each pulse. The noise is applied: (A) across the entire spectrum; (B) only to frequencies above 369 THz; and (C) as in B, but with mean-value shaping to eliminate the frequencies below 369 THz from the pulse spectrum. (Insets) Some detected pulse spectra. (D) SRS correlation spectra achieved by integrating the regions in A\u0026#x2013;C along the \u0026#x3C9;-axis indicated by the black dashed lines.\u0022 class=\u0022highwire-fragment fragment-images colorbox-load\u0022 rel=\u0022gallery-fragment-images-1831827155\u0022 data-figure-caption=\u0022\u0026lt;div class=\u0026quot;highwire-markup\u0026quot;\u0026gt;\u0026lt;div xmlns=\u0026quot;http:\/\/www.w3.org\/1999\/xhtml\u0026quot;\u0026gt;Covariance maps recorded in \u0026#x3B1;-quartz by applying uniform phase noise to each pulse. The noise is applied: (\u0026lt;em\u0026gt;A\u0026lt;\/em\u0026gt;) across the entire spectrum; (\u0026lt;em\u0026gt;B\u0026lt;\/em\u0026gt;) only to frequencies above 369 THz; and (\u0026lt;em\u0026gt;C\u0026lt;\/em\u0026gt;) as in \u0026lt;em\u0026gt;B\u0026lt;\/em\u0026gt;, but with mean-value shaping to eliminate the frequencies below 369 THz from the pulse spectrum. (\u0026lt;em\u0026gt;Insets\u0026lt;\/em\u0026gt;) Some detected pulse spectra. (\u0026lt;em\u0026gt;D\u0026lt;\/em\u0026gt;) SRS correlation spectra achieved by integrating the regions in \u0026lt;em\u0026gt;A\u0026lt;\/em\u0026gt;\u0026#x2013;\u0026lt;em\u0026gt;C\u0026lt;\/em\u0026gt; along the \u0026#x3C9;-axis indicated by the black dashed lines.\u0026lt;\/div\u0026gt;\u0026lt;\/div\u0026gt;\u0022 data-icon-position=\u0022\u0022 data-hide-link-title=\u00220\u0022\u003E\u003Cspan class=\u0022hw-responsive-img\u0022\u003E\u003Cimg class=\u0022highwire-fragment fragment-image lazyload\u0022 alt=\u0022Fig. 2.\u0022 src=\u0022data:image\/gif;base64,R0lGODlhAQABAIAAAAAAAP\/\/\/yH5BAEAAAAALAAAAAABAAEAAAIBRAA7\u0022 data-src=\u0022https:\/\/广东快乐十分投注下载 www.hmclip.net\/content\/pnas\/116\/12\/5383\/F2.medium.gif\u0022 width=\u0022440\u0022 height=\u0022150\u0022\/\u003E\u003Cnoscript\u003E\u003Cimg class=\u0022highwire-fragment fragment-image\u0022 alt=\u0022Fig. 2.\u0022 src=\u0022https:\/\/广东快乐十分投注下载 www.hmclip.net\/content\/pnas\/116\/12\/5383\/F2.medium.gif\u0022 width=\u0022440\u0022 height=\u0022150\u0022\/\u003E\u003C\/noscript\u003E\u003C\/span\u003E\u003C\/a\u003E\u003C\/div\u003E\u003C\/div\u003E\u003Cul class=\u0022highwire-figure-links inline\u0022\u003E\u003Cli class=\u0022download-fig first\u0022\u003E\u003Ca href=\u0022https:\/\/广东快乐十分投注下载 www.hmclip.net\/content\/pnas\/116\/12\/5383\/F2.large.jpg?download=true\u0022 class=\u0022highwire-figure-link highwire-figure-link-download\u0022 title=\u0022Download Fig. 2.\u0022 data-icon-position=\u0022\u0022 data-hide-link-title=\u00220\u0022\u003EDownload figure\u003C\/a\u003E\u003C\/li\u003E\n\u003Cli class=\u0022new-tab\u0022\u003E\u003Ca href=\u0022https:\/\/广东快乐十分投注下载 www.hmclip.net\/content\/pnas\/116\/12\/5383\/F2.large.jpg\u0022 class=\u0022highwire-figure-link highwire-figure-link-newtab\u0022 target=\u0022_blank\u0022 data-icon-position=\u0022\u0022 data-hide-link-title=\u00220\u0022\u003EOpen in new tab\u003C\/a\u003E\u003C\/li\u003E\n\u003Cli class=\u0022download-ppt last\u0022\u003E\u003Ca href=\u0022\/highwire\/powerpoint\/855377\u0022 class=\u0022highwire-figure-link highwire-figure-link-ppt\u0022 data-icon-position=\u0022\u0022 data-hide-link-title=\u00220\u0022\u003EDownload powerpoint\u003C\/a\u003E\u003C\/li\u003E\n\u003C\/ul\u003E\u003C\/div\u003E\u003Cdiv class=\u0022fig-caption\u0022 xmlns:xhtml=\u0022http:\/\/www.w3.org\/1999\/xhtml\u0022\u003E\u003Cspan class=\u0022fig-label\u0022\u003EFig. 2.\u003C\/span\u003E \u003Cp id=\u0022p-21\u0022\u003ECovariance maps recorded in \u03b1-quartz by applying uniform phase noise to each pulse. The noise is applied: (\u003Cem\u003EA\u003C\/em\u003E) across the entire spectrum; (\u003Cem\u003EB\u003C\/em\u003E) only to frequencies above 369 THz; and (\u003Cem\u003EC\u003C\/em\u003E) as in \u003Cem\u003EB\u003C\/em\u003E, but with mean-value shaping to eliminate the frequencies below 369 THz from the pulse spectrum. (\u003Cem\u003EInsets\u003C\/em\u003E) Some detected pulse spectra. (\u003Cem\u003ED\u003C\/em\u003E) SRS correlation spectra achieved by integrating the regions in \u003Cem\u003EA\u003C\/em\u003E\u2013\u003Cem\u003EC\u003C\/em\u003E along the \u03c9-axis indicated by the black dashed lines.\u003C\/p\u003E\u003Cdiv class=\u0022sb-div caption-clear\u0022\u003E\u003C\/div\u003E\u003C\/div\u003E\u003Cspan class=\u0022highwire-journal-article-marker-end\u0022\u003E\u003C\/span\u003E\u003C\/div\u003E\u003Cspan id=\u0022related-urls\u0022\u003E\u003C\/span\u003E\u003C\/div\u003E\u003C\/div\u003E\u003C\/div\u003E\u003C\/li\u003E\n\u003C\/ul\u003E\u003C\/div\u003E\u003C\/div\u003E\u003C\/div\u003E \u003C\/div\u003E\n\n \n \u003C\/div\u003E\n\u003Cdiv class=\u0022panel-separator\u0022\u003E\u003C\/div\u003E\u003Cdiv class=\u0022panel-pane pane-panels-mini pane-jnl-pnas-tab-supp\u0022 \u003E\n \n \n \n \u003Cdiv class=\u0022pane-content\u0022\u003E\n \u003Cdiv class=\u0022panel-display panel-1col clearfix\u0022 id=\u0022mini-panel-jnl_pnas_tab_supp\u0022\u003E\n \u003Cdiv class=\u0022panel-panel panel-col\u0022\u003E\n \u003Cdiv\u003E\u003Cdiv class=\u0022panel-pane pane-highwire-article-data-supp\u0022 \u003E\n \n \u003Ch2 class=\u0022pane-title\u0022\u003E\u003Cspan class=\u0022pane-title-text\u0022\u003EData supplements\u003C\/span\u003E\u003C\/h2\u003E\n \n \n \u003Cdiv class=\u0022pane-content\u0022\u003E\n \u003Cdiv class=\u0022item-list\u0022\u003E\u003Cul\u003E\u003Cli class=\u0022first last\u0022\u003E\u003Cdiv class=\u0022highwire-markup\u0022\u003E\u003Cdiv xmlns=\u0022http:\/\/www.w3.org\/1999\/xhtml\u0022 id=\u0022content-block\u0022 xmlns:xhtml=\u0022http:\/\/www.w3.org\/1999\/xhtml\u0022\u003E\u003Cdiv\u003E\u003Cspan class=\u0022highwire-journal-article-marker-start\u0022\u003E\u003C\/span\u003E\u003Cdiv class=\u0022auto-clean\u0022\u003E\u003Cspan style=\u0022font-family: Verdana,Arial,Helvetica,sans-serif; font-size: 83.33%\u0022\u003E\n \n \u003Ch2\u003ESupporting Information\u003C\/h2\u003E\n \u003Cul\u003E\u003Cli\u003E\u003Ca href=\u0022\/highwire\/filestream\/852015\/field_highwire_adjunct_files\/0\/pnas.1821048116.sapp.pdf\u0022 class=\u0022rewritten\u0022 data-icon-position=\u0022\u0022 data-hide-link-title=\u00220\u0022\u003EDownload Appendix (PDF)\u003C\/a\u003E \n \n \u003C\/li\u003E\u003C\/ul\u003E\n \u003C\/span\u003E\n \n \u003C\/div\u003E\u003Cspan class=\u0022highwire-journal-article-marker-end\u0022\u003E\u003C\/span\u003E\u003C\/div\u003E\u003Cspan id=\u0022related-urls\u0022\u003E\u003C\/span\u003E\u003C\/div\u003E\u003C\/div\u003E\u003C\/li\u003E\n\u003C\/ul\u003E\u003C\/div\u003E \u003C\/div\u003E\n\n \n \u003C\/div\u003E\n\u003C\/div\u003E\n \u003C\/div\u003E\n\u003C\/div\u003E\n \u003C\/div\u003E\n\n \n \u003C\/div\u003E\n\u003Cdiv class=\u0022panel-separator\u0022\u003E\u003C\/div\u003E\u003Cdiv class=\u0022panel-pane pane-earthchem\u0022 \u003E\n \n \n \n \u003Cdiv class=\u0022pane-content\u0022\u003E\n \u003Ca href=\u0022http:\/\/ecp.iedadata.org\/doidata\/10.1073\/pnas.1821048116\u0022 class=\u0022\u0022 data-icon-position=\u0022\u0022 data-hide-link-title=\u00220\u0022\u003E\u003Cimg src=\u0022http:\/\/ecp.iedadata.org\/doibanner\/10.1073\/pnas.1821048116\u0022 alt=\u0022\u0022 \/\u003E\u003C\/a\u003E \u003C\/div\u003E\n\n \n \u003C\/div\u003E\n\u003C\/div\u003E\n \u003C\/div\u003E\n\u003C\/div\u003E\n\u003C\/div\u003E\u003Cscript type=\u0022text\/javascript\u0022 src=\u0022https:\/\/广东快乐十分投注下载 www.hmclip.net\/sites\/default\/files\/js\/js_hZg96SP9gBcOluDp2mGc57d8sP8uJ7g8P_JYsCISOgQ.js\u0022\u003E\u003C\/script\u003E\n\u003C\/body\u003E\u003C\/html\u003E"}
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